Elektra's VP of A&R, Terry Tolkin, was impressed and Wareham signed a deal with Elektra, and started pulling together a band. He first contacted Justin Harwood, whom he had met while Harwood was playing with The Chills, and they recruited drummer Byron Guthrie, formerly from Ultra Vivid Scene. The trio recorded demos (produced by Dave Fridmann) and played a series of live dates with Mercury Rev guitarist Grasshopper. Guthrie was replaced by former Feelies drummer Stanley Demeski, and this line-up recorded the first album, Lunapark, produced by Fred Maher and released by Elektra under the name Luna² to avoid confusion with a new-age musician known as "Luna". (Later an accord was reached which allowed the band to use the name Luna.)
Shortly after the release of Lunapark, the band placed an advertisement in the Village Voice for a guitarist, and Canadian former drama student Sean Eden was recruited. The new four-piece recorded a number of cover versions that would become the Slide EP, and then toured the US. In mid-1993 the band supported the reformed Velvet Underground on their European tour, after which they recorded their second album. Bewitched was recorded in New York City and co-produced by the band with Victor Van Vugt. Velvet Underground guitarist Sterling Morrison played guitar on two tracks. The album was released in 1994.
In 1995, the band went into Sorcerer Sound studio in New York City with producer Pat McCarthy and engineer Mario Salvati to record their third album Penthouse. The album featured Television guitarist Tom Verlaine on the tracks "Moon Palace" and "23 Minutes in Brussels." The album was released in August 1995 to critical acclaim, with Rolling Stone declaring it one of the essential albums of the 1990s. The album featured a cover of Serge Gainsbourg's "Bonnie and Clyde" as a hidden track; the song featured Lætitia Sadier of Stereolab duetting with Dean Wareham. "Bonnie and Clyde" was released as a single in the UK and was named Melody Maker single of the week. Pup Tent followed in 1997.
In 1999, the band recorded The Days of Our Nights for Elektra, but the label declined the album as "not commercially viable" and dropped the band. The record was ultimately released on Jericho Records in the US. Prior to the album's release, Justin Harwood left the band, and was replaced by Britta Phillips. Phillips and Wareham began a romantic affair, leading to Wareham's divorce; the new couple eventually married.
After releasing Luna Live (2001), Romantica (2002) and Rendezvous (2004) with their new line-up, Luna announced their final tour (at the time), disbanding after a show at the Bowery Ballroom on February 27, 2005.
Dean Wareham and Britta Phillips continued on as the duo Dean & Britta, initially formed in 2003.
In 2012, Sean Eden joined a Dean & Britta performance at the Shine A Light Festival in Brooklyn, performing a short set of Luna tunes in a one-off reunion performance.
In 2014, Dean Wareham announced via Twitter that Luna would reunite for a tour of Spain in 2015, to be followed by US dates.
In 2017, Luna announced two new releases, a Luna covers LP, A Sentimental Education, and a 6-song original instrumental EP, A Place Of Greater Safety, with a tour of Spain in October and a North American tour in November 2017. Since then, Luna has been touring around the United States and Europe.
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